U. Baltensperger et al., AEROSOL CLIMATOLOGY AT THE HIGH-ALPINE SITE JUNGFRAUJOCH, SWITZERLAND, JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 102(D16), 1997, pp. 19707-19715
Continuous aerosol measurements have been performed at the high-alpine
site Jungfraujoch (3450 m above sea level) since 1988 by means of an
epiphaniometer. The instrument, which determines the Fuchs surface are
a of the aerosol particles, was operated with a time resolution of 30
min. High correlation coefficients (r > 0.8) were found between the ep
iphaniometer signal and other aerosol parameters, which could be attri
buted to a rather constant size distribution of the Jungfraujoch aeros
ol in the accumulation range (0.1 < d < 1 mu m). Well-defined diurnal
variations with a peak in the late afternoon were observed on many day
s during summer, which was not the case during winter. Comparison with
black carbon and radon daughter measurements revealed that these diur
nal variations are due to vertical transport processes. A statistical
analysis showed that the fraction of days with a well-defined diurnal
pattern increased with decreasing stability of the atmosphere; however
, late afternoon peaks also occurred during days when the potential te
mperature profile indicated a stable atmosphere. First simulations wit
h ALPTHERM, a new convection model which takes topography into account
, were able to explain the observed aerosol patterns. This indicates t
hat slope winds over a certain catchment area are responsible for the
transport to this high-elevation site. The distinct seasonal variation
with summer values, which are about a factor of 10 higher than winter
values, could therefore be attributed to seasonally varying transport
processes, due to the seasonal variation of radiation. The data show
that even sites at very high elevation cannot be assumed to be in the
free troposphere all the time.