Diffuse ultrahigh energy gamma radiation can arise from a variety of a
strophysical sources, including the interaction of 10(20) eV cosmic ra
ys with the 2.7 K microwave background radiation or the collapse of to
pological defects created in the early Universe. We describe a sensiti
ve search for diffuse gamma rays at ultrahigh energies using the Chica
go Air Shower Array-Michigan Muon Array experiment. An isotropic flux
of radiation is not detected, and we place stringent upper limits on t
he fraction of the gamma-ray component relative to cosmic rays (<10(-4
)) at energies from 5.7 x 10(14) to 5.5 X 10(16) eV. This result repre
sents the first comprehensive constraint on the gamma-ray flux at thes
e energies.