C. Boemare et al., OPTICAL STUDIES IN ZNSE GAAS EPILAYERS - FABRY-PEROT MODES IN THE UPPER BRANCH OF THE POLARITON/, Journal of crystal growth, 159(1-4), 1996, pp. 826-829
We report the observation of discrete modes in the upper branch of the
exciton-polariton. In micrometer thick ZnSe epilayers grown on GaAs s
ubstrates by metal organic vapour phase epitaxy we have studied the ev
olution of the reflectivity spectra as a function of the thickness of
the deposited ZnSe layers. For layer thickness in the range of a micro
n we observe reflectance oscillations that we interpret as due to Fabr
y-Perot modes in the upper branch of the polariton. This observation i
s possible due to the large exciton binding energy in ZnSe and the sub
sequent large energy extension of this branch. The amplitude of these
oscillations and their energy splitting decrease with increasing thick
ness of the epilayer. They could no longer be observed for thickness l
arger than 4.5 mu m. The effect is analyzed in the context of a semicl
assical approach using a non-local description of the dielectric const
ant, combined with results previously obtained in thin layers of bulk
CdSe and CuCl.