Hh. Wang et al., SUBPICOSECOND CARRIER RESPONSE OF UNANNEALED LOW-TEMPERATURE-GROWN GAAS VS TEMPERATURE, Journal of electronic materials, 22(12), 1993, pp. 1461-1464
The subpicosecond carrier lifetime of an unannealed molecular beam epi
taxial layer of GaAs grown at similar to 210 degrees C has been demons
trated between 10 and 290K through optoelectronic switching and all-op
tical pump-probe measurements. The low room-temperature resistivity of
the as-grown layers, believed to arise from hopping conductivity thro
ugh defect sites, has been observed to increase as the sample temperat
ure was lowered, allowing ultrafast switching measurements to be perfo
rmed using the low-temperature-as-grown GaAs as a photoconductive elem
ent. After illumination by 100 femtosecond optical pulses, photogenera
ted carriers in the sample have rapidly relaxed, returning the materia
l to its high-resistivity state in less than 1 ps. This indicates that
the precipitates present in post-annealed samples are not required fo
r the fast relaxation of photoexcited carriers in low-temperature-grow
n GaAs. Ultrafast switching measurements on a post-annealed version of
the GaAs film also resulted in the generation of similar, 0.6 ps full
width at half maximum pulses.