NEUTRINO-RECOIL INDUCED DESORPTION

Citation
L. Zhu et al., NEUTRINO-RECOIL INDUCED DESORPTION, Journal of vacuum science & technology. A. Vacuum, surfaces, and films, 12(4), 1994, pp. 2037-2044
Citations number
17
Categorie Soggetti
Physics, Applied","Materials Science, Coatings & Films
ISSN journal
07342101
Volume
12
Issue
4
Year of publication
1994
Part
2
Pages
2037 - 2044
Database
ISI
SICI code
0734-2101(1994)12:4<2037:NID>2.0.ZU;2-V
Abstract
Nuclear decay induced Cl-37 ion desorption from the electron capture d ecay Ar-37-->Cl-37+nu is reported for the first time. A mixture of one part Ar-36 and approximately 5X10(-5) parts Ar-37 (Ar-36/37) is physi sorbed on a gold-plated Si wafer kept at 16 K under ultrahigh vacuum c onditions. The time of flight (TOF) of recoiled Cl-37 ions is measured using coincidence techniques. The observed kinetic energy distributio n of the Cl-37 ions is approximately Gaussian in shape, with a maximum at almost-equal-to 9.0 eV and a full width at half-maximum of approxi mately 3 eV. Considering the binding energy of physisorbed Ar-37 is ap proximately 80 meV, the 9-eV peak energy compares well with that of th e gas-phase value, where conservation of the energy and momentum fixes the kinetic energy of Cl-37 ions at 9.54 eV. Using a combination of T OF and retarding field energy analysis, the charge states of detected ions for 1 ML (monolayer) of Ar-36/37 are determined as 53%+1e, 21%+2e , and 26%+ne, where n greater-than-or-equal-to 3. The fraction of deca ying Ar-37 atoms which emerge from the surface as positive Cl-37 ions is found to be 10%. Finally, a strong charge exchange reaction between a Cl-37 ion and near-neighbor atoms causes a Coulomb explosion within the multilayers, increasing the kinetic energy of desorbing ions by a s much as approximately 7 eV.