Ad. Bekkerman et al., FRAGMENTATION OF SPUTTERED CLUSTER IONS OF TRANSITION-METALS - DISTRIBUTIONS OF LIFETIMES AND INTERNAL ENERGIES, Mikrochimica acta (1966), 1998, pp. 371-377
Dissociation energies, lifetime distributions and internal energies ha
ve been determined experimentally for Fe-n(+) (4 less than or equal to
n less than or equal to 10) clusters produced by sputtering under 8.5
keV Xe+ ion bombardment. The average lifetimes and the average intern
al energies were calculated from the experimental distributions. A com
parison between the results of the present work on Ta-n(+) and Nb-n(+)
clusters and those obtained earlier has been made. For all sputtered
clusters compared, the linear dependence of the average internal energ
y (E) over bar(int) on the number of atoms, n, in the cluster has been
identified. Good qualitative agreement has been found between experim
ental results and theoretical values determined from MD-simulations of
cluster sputtering processes.